WSI dev: Research overview

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title => protected'Brandt Group' (12 chars)

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description => protected'Our research addresses new semiconductor materials and n
ew spectroscopic methods for their characterization. For qu
antum information processing, we develop new tools based on magnetic resonan
ce which allow to manipulate and detect the spin state of quantum bits via e
lectrical transport measurements. As qubits, we in particular study the nucl
ear spins of ionized donors, which based on our pioneering work have been de
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re, by far exceeding any other solid-state-based qubit system.' (598 chars)

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title => protected'Prof. Dr.' (9 chars)

description => protected'Martin Brandt is a Professor at the Walter Schottky
Institut and at the Physik-Department of the Technische Universität München
in Garching, Germany. After studying physics at Universität Bonn, University
of Oxford and TU München, he joined the group of Manuel Cardona at the Max-
Planck-Institut für Festkörperforschung and received his Dr. rer. nat. degre
e from Universität Stuttgart in 1992. In 1993, he was a postdoc at Xerox Pal
o Alto Research Center supported by a Feodor Lynen fellowship of the Alexand
er von Humboldt foundation. Also that year, Martin Brandt was awarded the Ot
to-Hahn-Medal of the Max-Planck-Society. In 1994, he joined the Schottky Ins
titut, where he became Privatdozent in 1999 and was appointed außerplanmäßig
er Professor in 2006. His work focuses on the physics and applications of do
pants and defects in semiconductors, including silicon, diamond, nitrides an
d oxides. The main research tool of his group is magnetic resonance, spearhe
ading the development of alternative detection methods such as via electroni
c transport measurements to increase the sensitivity of this type of spectro
scopy. Martin Brandt has published more than 250 papers, mostly in peer-revi
ewed journals, and holds 16 patents. He has been a member of the DFG-funded
Collaborative Research Centers 348, 563 and 631 and of the Research Unit 149
3 “Diamond Materials for Quantum Applications”. Furthermore, he was initiato
r and member of the Priority Program 1602 “New Frontiers in Sensitivity for
EPR Spectroscopy”. Currently, Martin Brandt is a core member of the Munich C
enter for Quantum Science and Technology. He is a member of the editorial bo
ard of the journal physica status solidi and has served on numerous conferen
ce program committees, including chairing the 2016 Gordon Conference on Defe
cts in Semiconductors.' (1850 chars)

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shortdescription => protected'Photonic and optoelectronic phenomena on the nanometer scale are at the hear
t of fundamental science and technology. The institute explores various opto
electronic systems.' (171 chars)

description => protected'Photonic and optoelectronic phenomena on the nanometer scale are at the h
eart of fundamental science and technology. The institute explores various o
ptoelectronic systems.' (178 chars)

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shortdescription => protected'In the WSI, we develop new semiconductors, catalytic assemblies, and nanosys
tems that are the engines of advanced energy conversion devices.' (140 chars)

description => protected'Renewable energy harvesting and efficient energy utilization are essentia
l for creating a sustainable future. In the WSI, we develop new semiconducto
rs, catalytic assemblies, and nanosystems that are the engines of energy con
version devices, including solar fuels generators, photovoltaics, and solid
state lighting. Advanced microscopic and spectroscopic characterization meth
ods provide mechanistic insights that guide new strategies for fabrication o
f functional systems offering improved stabilities and efficiencies.' (528 chars)

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title => protected'Widely-tunable room-temperature THz quantum cascade laser sources' (65 chars)

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shortdescription => protected'THz spectral range is teeming with mainstream concepts. However, it is st
ill in need of a convenient and compact semiconductor source and detector te
chnology. In particular, THz radiation sources are bulky, complex in operati
on, and expensive to manufacture. Real-world applications require room-te
mperature broadly-tunable or frequency-comb THz sources that are similar
in operation simplicity and mass producibility to diode lasers and mid-IR q
uantum cascade lasers (QCLs). We have recently achieved significa
nt progress in the development of such sources [1,2]. Our devices are based
on efficient frequency mixing inside of dual-wavelength mid-IR QCLs. Their a
ctive regions are quantum-engineered to provide a giant nonlinearity for dif
ference-frequency generation (DFG) with population inversion [1,2] and their
waveguides are designed for Cherenkov phase-matching of DFG that enables TH
z extraction through the substrate [3]. As a result, these devices (referred
to as THz DFG-QCLs) can now provide up to nearly 2 mW of peak THz power out
put and over 10 µW of continuous-wave THz power at room temperature [1,2]. A
schematic of a Cherenkov THz DFG-QLC is shown in the figure on the right.&n
bsp;' (1224 chars)

description => protected'A typical single mode device performance is shown in Fig. 1(a). We have a
lso demonstrated that THz DFG-QCL chips can be continuously tuned over nearl
y the entire 1-6 THz range using an external cavity setup [3-5] or in monoli
thic configurations [6,7], see Fig. 2(b). We have further recently confirmed
that, in continuous-wave operation, these devices provide a narrow (sub-MHz
) emission linewidth which makes them suitable to be used as local oscillato
rs for heterodyne spectroscopy [8]. The THz DFG-QCL platform holds a high pr
omise for developing efficient broadband THz frequency comb sources for spec
troscopic and metrological applications. Our ongoing work is aime
d at improving the THz radiation outcouping efficiency (estimated to be belo
w ~5% in the current devices) [9,10], enhancing the optical nonlinearity in
the QCL active regions to increase THz output power, improving device therma
l packaging, generating THz frequency combs, developing miniature broadly-tu
nable THz systems, and demonstrating compact semiconductor-based THz instrum
entation such as spectroscopy and imaging systems, dual-comb spectrometers,
and microscopy systems.' (1167 chars)

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paragraph2 => protected'REFERENCES <ol><li>K. Fujita, S. Jung, Y. Jiang,
J.H. Kim, A Nakanishi, A. Ito, M. Hitaka, T. Edamura, and M.A. Belkin, “Rec
ent progress in terahertz difference-frequency quantum cascade laser sources
,” Nanophoton. 7, 1795-1817 (2018).</li><li>M.A. Bel
kin and F. Capasso, “New frontiers in quantum cascade lasers: high performan
ce room temperature terahertz sources,” Phys. Scr. 90, 118002 (2015).</li><li>K. Vijayraghavan, Y. Jiang, M. Jang, A. Jiang, K.
Choutagunta, A. Vizbaras, F. Demmerle, G. Boehm, M. C. Amann, and M. A. Belk
in, “Broadly tunable terahertz generation in mid-infrared quantum cascade la
sers,” Nature Commun. 4, 2021 (2013).</li><li>Y. Jia
ng, K. Vijayraghavan, S. Jung, F. Demmerle, G. Boehm, M.-C. Amann, and M.A.
Belkin “External cavity terahertz quantum cascade laser sources based on int
racavity frequency mixing with 1.2-5.9 THz tuning range,” J. Opt. <st
rong>16, 094002 (2014).</li><li>Y. Jiang, K. Vijayraghavan, S. Jung
, A. Jiang, J.H. Kim, F. Demmerle, G. Boehm, M.C. Amann, and M.A. Belkin, “S
pectroscopic study of terahertz generation in mid-infrared quantum cascade l
asers,” Sci. Rep. 6, 21169 (2016).</li><li>S. Jung,
A. Jiang, Y. Jiang, K. Vijayraghavan, X. Wang, M. Troccoli, and M.A. Belkin,
“Broadly tunable monolithic room-temperature terahertz quantum cascade lase
r sources,” Nature Commun. 5, 4267 (2014).</li><li>A
. Jiang, S. Jung, Y. Jiang, K. Vijayraghavan, J. Kim, and M.A. Belkin, “Wide
ly tunable terahertz source based on intra-cavity frequency mixing in quantu
m cascade laser arrays,” Appl. Phys. Lett. 106, 2611
07 (2015).</li><li>L. Consolino, S. Jung, A. Campa, M. De Regis, S. Pal, K.
Fujita, A. Ito, M. Hitaka, S. Bartalini, P. De Natale, M.A. Belkin, and M.S.
Vitiello, “Spectral purity and tunability of terahertz quantum cascade lase
r sources based on intra...' (2573 chars)

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title => protected'Integrated mid-infrared photonics' (33 chars)

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shortdescription => protected'Near-infrared (wavelengths approximately in the range of 1-2.5 microns) p
hotonic integrated circuits (PICs) based on the silicon-on-insulator (SOI) o
r III-V platforms have undergone a tremendous expansion in recent years, dri
ven initially by applications in fiber-optics communications and optical int
erconnects and later expanding to beam combining and steering, chemical and
biological sensing, and frequency comb generation. Near-infrared PIC systems
are now commercialized for several different applications by companies such
as Infinera, Sisco Systems, SICOYA, and many others. In contrast
to the near-infrared spectral range, mid-IR laser-based systems have so far
been designed around free-space optics. Integration of a semiconductor lase
r with a suitable mid-IR photonics platform will enable the development of m
id-IR PICs for a wide range of applications from spectroscopy and sensing to
beam steering aund ab nd new frequency generation. We have recently started
investigating approaches for developing mid-IR PICs using both silicon and
III-V platforms.' (1084 chars)

description => protected'Figure 2(a) shows the electron microscope image of a mid-IR QCL epi-trans
ferred to Silicon-on-Sapphire (SOS) wafers using 250-nm-thick SU-8 epoxy as
an adhesive. Efficient coupling of mid-IR light from the laser cavity to sil
icon waveguides was achieved using tapered QCL waveguides as shown in Fig. 3
(a) after Ref. [1]. Similar transfer-printing methods can be used to integra
te other mid-IR light sources, such as diode lasers and interband cascade la
sers (ICLs) with silicon waveguides. Hybrid mid-IR systems based
on III-V laser materials transferred to silicon photonic waveguides are expe
cted to perform well with mid-IR diode lasers and ICLs that have relatively
low (few tens of milliwatts) optical powers and thermal power dissipation. H
owever, long-wavelength room-temperature operation of these devices is limit
ed to the 5-6 microns spectral range. In addition, the use of the Si-based p
latforms limits the spectral range of mid-IR PICs to below 7 μm due to optic
al absorption in Si. QCLs are currently the only room-temperature
electrically pumped semiconductor light sources that can operate in the ent
ire mid-IR range (from 3 to 15 microns) with optical powers over 1 W. Given
the very high thermal dissipation in QCL active regions, achieving long-term
reliability and continuous-wave operation of heterogeneously integrated dev
ices on silicon platforms is challenging. Therefore, we have recently starte
d working on homogeneous integration of mid-IR QCLs with low-loss III-V pass
ive waveguides epitaxially grown on InP substrates, see Fig. 2(b). The homog
eneous integration approach uses materials, growth, and processing steps nea
rly identical to those used for conventional high-performance mid-IR QCLs, w
hich offers superior reliability and performance of photonic integrated circ
uits. Devices integrated with III-V waveguides show more than an order of ma
gnitude higher output power from passive waveguides, compared to devices int
egrated with the SOS wav...' (2275 chars)

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paragraph2 => protected'REFERENCES <ol><li>S. Jung, J. Kirch, J.H. Kim,
L.J. Mawst, D. Botez, and M.A. Belkin, “Quantum cascade lasers transfer-prin
ted on silicon-on-sapphire,” Appl. Phys. Lett. 111,
211102 (2017).</li><li>S. Jung, D. Palaferri, K. Zhang, F. Xie, Y. Okuno, C.
Pinzone, K. Lascola, and M.A. Belkin, “Homogeneous photonic integration of
mid-infrared quantum cascade lasers with low-loss passive waveguides on InP
platform,” Optica 6, 1023-1030 (2019).</li></ol>' (528 chars)

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title => protected'Quantum-engineered nonlinear metamaterials' (42 chars)

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shortdescription => protected'The mid-IR and THz regions are particularly suitable for creating enginee
red materials based on the concepts of quantum-engineering of electron state
s, plasmonics, and metamaterials. We have recently demonstrated the potentia
l of this approach by creating large-area ultrathin metasurfaces with record
-high nonlinear optical response. The metasurfaces operate by coupling modes
in electromagnetically-engineered plasmonic nanoresonators with quantum-eng
ineered intersubband nonlinearities in a thin semiconductor heterostructure.
 Subwavelength thickness of our metasurfaces precludes phase matc
hing constrains associated with traditional nonlinear optical crystals and t
hus allows for broadband frequency conversion. Furthermore, since very low o
ptical intensity is required to produce strong nonlinear effects, our metasu
rfaces may be pumped using compact continuous-wave semiconductor lasers such
as QCLs or diode lasers. Continuously-pumped metasurfaces may be used, for
example, to achieve self-referencing and frequency shift of low-power micror
esonator-based optical frequency comb sources to anywhere in mid-IR and THz,
to generate large amounts of THz radiation using high-power mid-IR pump las
ers (e.g., CO2 lasers or high-power QCLs), and to up-convert mid-
IR and THz optical signals for focal-plane-array imaging.' (1353 chars)

description => protected'The basic schematic of the metasurface is given in Fig. 4 and its operati
on is explained in the figure caption. We achieved over 0.075 % of mid-IR se
cond-harmonic power conversion efficiency using only 15 kW/cm2 of
pump intensity [1,2]. The second-order nonlinear susceptibility of our late
st metasurfaces at low pump intensity is estimated to be over 106
pm/V, 4 orders of magnitude higher than that of traditional nonlinear mater
ials such as LiNbO3. From the fundamental standpoint, our metasurfaces provi
de the foundation for the “flat nonlinear optics paradigm” in which we can s
imultaneously produce high nonlinear conversion efficiency and achieve full
control of the wavefront of the nonlinear output, as demonstrated by us in R
ef. [3]. We are now investigating numerous directions in which th
e effective nonlinearity and conversion efficiency of the metasurfaces may b
e further improved, particularly, by optimizing plasmonic nanoresonator desi
gns to achieve higher field enhancement and higher nonlinear overlap integra
l [4,5] and by increasing the intersubband nonlinearity and saturation inten
sity of the semiconductor heterostructure using more sophisticated MQW desig
ns. Theoretical simulations indicate that up to 10% of power conversion effi
ciency is possible in fully-optimized structures using input intensities ~10
-100 kW/cm2. Additional ongoing and planned future research on th
is topic include   <ul><li>Design and experimental test
ing of metasurfaces for THz difference-frequency generation [6];</li><li>Met
asurfaces for efficient up-conversion of mid-IR and THz signals for detectio
n and imaging;</li><li>Nonlinear metasurfaces for mid-IR and THz Raman lasin
g and other four-wave mixing processes such as phase conjugation and all-opt
ical control;</li><li>Investigating quantum effects in individual highly-non
linear nanoscale optical resonators [7].</li></ul>' (1950 chars)

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paragraph2 => protected'REFERENCES <ol><li>J. Lee, M. Tymchenko, C. Argy
ropoulos, P. Y. Chen, F. Lu, F. Demmerle, G. Boehm, M. C. Amann, A. Alu, and
M.A. Belkin, “Giant nonlinear response from plasmonic metasurfaces coupled
to intersubband transitions,” Nature 511, 65 (2014).
</li><li>J. Lee, N. Nookala, J. S. Gomez-Diaz, M. Tymchenko, F. Demmerle, G.
Boehm, M.-C. Amann, A. Alù, and M.A. Belkin “Ultrathin second-harmonic meta
surfaces with record-high nonlinear optical response,” Adv. Opt. Mat.
4, 664-670 (2016).</li><li>N. Nookala, J. Lee, J.S. Gomez-
Diaz, M. Tymchenko, F. Demmerle, G. Boehm, K. Lai, G. Shvets, M.-C. Amann, A
. Alù, and M.A. Belkin, “Ultrathin gradient nonlinear metasurface with a gia
nt nonlinear response,” Optica 3, 283-288 (2016).</l
i><li>N. Nookala, J. Xu, O. Wolf, S. March, R. Sarma, S. Bank, J. Klem, I. B
rener, and M. A. Belkin, “Mid-infrared second-harmonic generation in ultra-t
hin plasmonic metasurfaces without a full-metal backplane,” Appl. Phys. B
. 124, 132 (2018).</li><li>R. Sarma, D. de Ceglia, N. N
ookala, M. Vincenti, S. Campione, O. Wolf, M. Scalora, M. Sinclair, M. Belki
n and I. Brener, "Broadband and efficient second-harmonic generation from a
hybrid dielectric metasurface/semiconductor quantum-well structure," ACS
Photon. 6, 1458 (2019).</li><li>M. Tokman, Z. Long, S.
Al Mutairi, Y. Wang, V. Vdovin, M. Belkin, and A. Belyanin, “Purcell enhance
ment of the parametric down-conversion in two-dimensional nonlinear material
s,” APL Photonics 4, 034403 (2019).</li><li>M. Tymch
enko, J. S. Gomez-Diaz, J. Lee, M.A. Belkin, and A. Alù, “Highly-efficient T
Hz generation using nonlinear plasmonic metasurfaces,” J. Opt. <stron
g>19, 104001 (2017).</li></ol>' (1863 chars)

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title => protected'Mid-infrared vertical cavity surface emitting lasers (VCSELs)' (61 chars)

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shortdescription => protected'Gas sensing based on direct laser diode absorption spectroscopy is one of
the most sensitive and selective detection methods and it is widely used in
industry. Because of their geometry, vertical cavity surface emitting laser
s (VCSELs) are known to have significant advantages over edge-emitting diode
lasers, including extreme compactness, about two orders of magnitude lower
power consumption (due to smaller active region volume), round (rather than
elliptical) beam shape, and intrinsic single-mode operation without the need
for complex distributed feedback gratings used in single-mode edge-emitting
lasers (due to much smaller laser cavity size). Mid-IR spectral
range is often called the ‘molecular fingerprint region’ because any chemica
l compound can be uniquely described by its molecular absorption fingerprint
. The development of continuous-wave (CW) mid-IR VCSELs is highly desired fo
r the creation of compact chemical sensors with high detectivity and specifi
city. Currently, however, such VCSELs do not exist. We are working on the de
velopment of CW room-temperature mid-IR VCSELs in the wavelength range 3-5 µ
m.' (1146 chars)

description => protected'Due to current unavailability of CW VCSELs operating in the wavelength ra
nge of the fundamental molecular roto-vibrational absorption lines, devices
operating at shorter near-infrared (near-IR) wavelengths (often around 1550
nm) are used to target the absorption lines corresponding to “overtones” (hi
gher-order harmonics) of fundamental molecular vibrations. However, these li
nes are typically about 2 orders of magnitude weaker than the fundamental ab
sorption lines. Figure 5(a) shows the absorption spectrum of methane display
ing both fundamental absorption lines around 3300 nm and overtone lines
at 1550 nm and 2300 nm. Additionally, the overtone line spectrum of molecul
ar compounds is more complex and spectrally dense compared to the spectrum o
f the fundamental lines. As a result, it is often difficult to select an ove
rtone absorption line of a target molecule that is free from interference pr
oduced by overtone lines of other gases. Our research efforts foc
us on developing CW room-temperature mid-IR VCSELs operating in the 3-5 µm w
avelength range using InAlGaAsSb heterostructures grown on GaSb substrates.
The schematic of a VCSEL structure is shown in Fig. 5(b). The Chair has prod
uced devices that define the current state of the art in the mid-IR VCSEL te
chnology, including CW VCSELs at 3 µm wavelength [1] and at 4 µm wavelength
[2] with near-room-temperature operation, see Fig. 6. Current res
earch efforts are focused on improving the active region design of the devic
es using both type-I and type-II active region schemes, improving the mirror
design and the current injection aperture design in these devices, optimizi
ng thermal packaging and more. The development of the first CW mid-IR VCSELs
is also expected to lead to various opportunities in application of these d
evices for gas sensing and spectroscopy.' (1868 chars)

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paragraph2 => protected'REFERENCES <ol><li>A. Andrejew, S. Sprengel, and
M.-C. Amann, "GaSb-based vertical-cavity surface-emitting lasers with an em
ission wavelength at 3 μm", Opt. Lett. 41, 2799 (201
6).</li><li>G.K. Veerabathran, S. Sprengel, A. Andrejew, and M.-C. Amann, "R
oom-temperature vertical-cavity surface-emitting lasers at 4 μm with GaSb-ba
sed type-II quantum wells", Appl. Phys. Lett. 110, 0
71104 (2017).</li></ol>' (479 chars)

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title => protected'Finley Group' (12 chars)

descriptivename => protected'Semiconductor Nanostructures and Quantum Systems (SNQS)' (55 chars)

description => protected'Semiconductor Nanostructures and Quantum Sys
tems (SNQS) A very warm welcome to the
chair for Semiconductor Nanostructures and Quantum Systems (SN
QS) at the Walter Schottky Institute&nbs
p;of the Technical University of Munich. We perform cu
tting-edge research and teaching in experimental condensed matter ph
ysics, with a particular focus on emergent quantum material
s based on semiconductors, the development of advanced spec
troscopic tools, and the exploration of novel quantum phase
s of matter.' (709 chars)

description2 => protected'Quantum Materials & Epitaxy: We
synthesise a wide range of quantum nano-materials, including group-III arse
nide and antimonide semiconductors as well as atomically thin 2D materials.
Material growth uses molecular beam epitaxy (MBE) systems, equipped with adv
anced in-situ diagnostics. These include low-temperature optical spec
troscopy performed inside the UHV environment, enabling real-time characteri
sation of material properties. Strongly
Correlated 2D Quantum Systems: We explore heterostructures formed
by stacking van der Waals materials, where strong charge and spin correlatio
ns lead to rich optical, electronic, and magnetic phenomena. Our research fo
cuses on probing such correlated quantum states, with the goal of discoverin
g and exploring new quantum states of matter.   Quantum Photonics & Light–Matter Interactions: We
develop quantum photonic technologies, including sources of entangled photo
ns for quantum communication and computation. Working closely with the QEC g
roup led by <a href="https://www.ee.cit.tum.de/qec/home/">Kai Müller at T
UM-CIT</a> we also study fundamental aspects of light–matter interaction
in such systems. In partnership with <a href="https://munich-quantum-instru
ments.com/">Munich Quantum Instruments</a> GmbH, we work on supercond
ucting single-photon detectors. Group-I
V Quantum Emitters: We develop hexagonal SiGe quantum heterostructu
res in an ERC Synergy project with <a href="https://www.tue.nl/en/research/r
esearch-groups/advanced-nanomaterials-devices">Erik Bakkers (TU Eindhoven
)</a> and <a href="https://www.utwente.nl/en/eemcs/ne/">Floris Zwanen
burg (University of Twente)</a>. Hex-SiGe has a direct bandgap, opening
exciting possibilities for group-IV nanolasers, quantum light sources, and s
pin–photon interfaces.</...' (2399 chars)

description3 => protected'' (0 chars)

description4 => protected'We are always interested to hear from highly motivated undergraduates, Ph
D-candidates and postdocs who might be interested in joining our laboratorie
s. Please send an email to <a class="group_submenu" href="mailto:jj.finley@t
um.de" target="new_mail">Jonathan Finley</a> with a copy of your CV and a br
ief (10 line) motivation for joining us.' (348 chars)

description5 => protected'We very gratefully acknowledge third-party funding for the research condu
cted at SNQS – it supports a lot of talented postdocs, grad and undergraduat
e students and creates an environment that makes science enjoyable for all o
f us!' (237 chars)

description6 => protected'Our funding sources include the German Science Foundation (DFG) via vario
us individual projects and we are proud members of the DFG Excellence Cluste
rs (<a href="http://mcqst.de/" target="_blank">MCQST</a>) and <a href="https
://www.e-conversion.de/" target="_blank">e-conversion</a>. Other major resea
rch efforts include the German Federal Ministry of Education and Research (B
MBF), the European Union (EU) via Horizon 2020 and the Quantum Flagship, the
Bavarian Science Ministry (ExQM), the Max-Planck-Society (IMPRS), the Inter
national Graduate school of Science and Engineering (IGSSE), the TUM Institu
te of Advanced Study (TUM-IAS) and various industrial partners. We were deli
ghted that Gregor Koblmüller was successful in his application for the prest
igious ERC Consolidator Grant.' (794 chars)

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shortdescription => protected'Underlying almost all of the science we do at SNQS is the availability of
precise nanostructures created by design using controlled synthesis methods
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des and, most recently, ultra-pure 2D materials and their heterostructures.
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description => protected'<div class="abstract">Underlying almost all of the science we do at SNQS
is the availability of precise nanostructures created by design using contro
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ides), group-III nitrides and, most recently, ultra-pure 2D materials and th
eir heterostructures. Currently, a substantial effort in synthesis is on III
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paragraph2 => protected'Underlying almost all of the science we do at SNQS is the availability of
precise nanostructures created by design using controlled synthesis methods
. We employ high-purity molecular beam epitaxy (MBE) dedicated to III-V comp
ound semiconductors (group-III arsenides & antimonides), group-III nitri
des and, most recently, ultra-pure 2D materials and their heterostructures.
Currently, a substantial effort in synthesis is on III-V nanowires (NW), whi
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g, as well as site-selective growth and deterministic incorporation of atomi
cally engineered low-dimensional quantum systems. <div class="abstract"
>Underlying almost all of the science we do at SNQS is the availability o
f precise nanostructures created by design using controlled synthesis method
s. We employ high-purity molecular beam epitaxy (MBE) dedicated to III-V com
pound semiconductors (group-III arsenides & antimonides), group-III nitr
ides and, most recently, ultra-pure 2D materials and their heterostructures.
Currently, a substantial effort in synthesis is on III-V nanowires (NW), wh
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ng, as well as site-selective growth and deterministic incorporation of atom
ically engineered low-dimensional quantum systems.</div>' (1352 chars)

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shortdescription => protected'Semiconductor lasers promise to have improved performance and novel prope
rties as their physical size is scaled down to the quantum limit for electro
ns and photons. One of the major research directions at SNQS focuses on deve
loping high-performance integrated (quantum)photonic and optoelectronic devi
ces based on monolithically integrated nanowires (NWs). Specific examples in
clude NW-based lasers and non-classical single photon emitters based on NW-Q
D devices. Hereby, an important task is to explore the optical and photonic
responses of the respective systems using advanced confocal luminescence spe
ctroscopy, where e.g. the effects of the quantized electronic structure, lig
ht-matter interactions, or the coupling of light to on-chip photonic circuit
s are explored.' (779 chars)

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shortdescription => protected'Superlattices are artificial, periodic potentials wh
ich are used to confined particles and quasiparticles such as atoms, electro
ns, or excitons. If the trapped quasiparticles are allowed to interact, the
resulting many-body state can capture essential behaviors of canonical quant
um many-body theories (e.g. the Hubbard model). Such artificial quasiparticl
e lattices are often called analogue quantum simula
tors. A bit like a quantum wind tunnel, the quantum simulator serve
s as an engineerable scale model of a real physical system (electrons or oth
er particles in a real crystalline solid) which allows us to probe complicat
ed many-body physics with a high level of control. Such many-body physics ar
e often hard to describe or predict theoretically, so our quantum simulators
provide a route to benchmark leading theories and discover new phases of ma
tter beyond current theoretical predictions.' (960 chars)

description => protected'Our approach to quantum simulation is to create supe
rlattices in 2D semiconductors by engineering an artificial electrostatic po
tential. This is accomplished by applying a bias voltage between a monolayer
semiconductor and a nearby thin graphite layer which has been patterned wit
h a periodic array of holes, generating a periodic potential/electric field
profile in the 2D semiconductor layer which can trap charges. The depth of t
he superlattice potential can be easily tuned, and any lattice geometry can
be implemented due to our top-down fabrication approach. We probe the superl
attice devices using a combination of optical spectroscopy, relying on the n
atural sensitivity of the optically-active excitons to the correlated behavi
or of the charges in the superlattice, complemented by charge transport meas
urements.   ' (897 chars)

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title => protected'Neuromorphic Photonic Systems' (29 chars)

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shortdescription => protected'Besides their spectacular optical, spin and electronic properties 2D mate
rials can also exhibit ferroelectric order that arises as a consequence of t
he stacking order of van-der-Waals (vdW) layered materials and polarisation
fields that emerge within the unit cell of the crystal.  Such ferroelec
tricity can be controlled by strain & sliding of the component vdW layer
s of the materials.  We explore high-quality 3R-stacked polytypes of TM
Ds that exhibit out-of-plane ferroelectricity.  In 3R-TMD bilayers, sli
ding one monolayer a few Ångströms over the other flips the ferroelectric po
larisation, a new ‘slidetronics’ concept in condensed matter physics inspire
d by twistronics.  Such materials are deal for nanoscale systems in whi
ch ferroelectric order can be controlled with light, providing exciting new
opportunities for optoelectronics, neuromorphic photonics, and sensing.
' (917 chars)

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title => protected'2D Magnetic Semiconductors' (26 chars)

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shortdescription => protected'The chromium chalcogen halides (CrXH) are an emerging family of 2D semico
nductors with a direct bandgap, highly anisotropic structural and electronic
properties, and robust magnetic order with ordering temperatures up to room
temperature. We seek to understand and engineer interactions between the ma
gnetic order in CrXH compounds and the excitons they host. The unique magnet
ic and optical properties of CrXH materials present unique opportunities to
develop spintronic devices with magnetic and optical controllability.' (529 chars)

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dictum, vulputate tortor vitae, placerat dui. Pellentesque cursus ultricies
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dio.' (1224 chars)

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title => protected'Van der Waals Materials for Integrated Nanophotonics' (52 chars)

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shortdescription => protected'Integrated quantum photonics is pivotal for the impl
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ton sources and diverse components, such as waveguides, beam splitters, inte
rferometers etc. required for steering and processing the quantum signals pr
oduced by the sources. In order to insure performance stability, as well as
to minimise energy consumption, photonic circuits should integrate as many c
omponents as possible on a same chip. To this respect, a critical hurdle is
represented by the necessity to assemble different materials that accomplish
different tasks. In the <a href="https://cordis.europa.eu/project/id/101186
642">VALERIA project</a> our long term vision is to realise a single-materia
l photonic platform exploiting the nano-structuring of transition metal dich
alcogenides. The demonstration of this vision will be the fabrication of all
-in-one devices made of a single TMD bulk crystal embedding site-controlled
single photon emitters integrated with photonic crystal cavities and coupled
to waveguides, beamsplitters amd non linear optical components.  ' (1215 chars)

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title => protected'Artificial Molecules as Spin-Photon Interfaces' (46 chars)

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shortdescription => protected'III-V quantum dots (QDs) host ultrastable spin-qubits that can be optical
ly addressed. They are used as deterministic and highly efficient sources of
single photons, entangled photon pairs and streams of polarisation entangle
d photons for quantum photonic technologies.  Single spins can create t
imed strings of entangled photons. Pairs of tunnel coupled spins in QD-molec
ules can be used to generate non-classical states of light with 2D entanglem
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echnologies.  ' (555 chars)

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title => protected'Quantum Transduction' (20 chars)

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shortdescription => protected'A quantum transducer converts quantum information betwee
n different physical systems, such as photons, phonons, or spins. It enables
communication across platforms that operate at distinct, and frequently dis
parate frequency or energy scales.  Such devices are essential for link
ing quantum processors to long-distance quantum communication networks. &nbs
p;Working as part of the <a href="https://www.munich-quantum-valley.de">Muni
ch Quantum Valley</a> project, WSI groups are working on the development of
high bandwidth, semiconductor based quantum transducer modules capable of ef
ficiently mapping between microwave quantum states of light and photons in t
he telecommunications band that can be distributed over optical fibers. &nbs
p;' (766 chars)

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title => protected'Superconducting Nanowire Single Photon Detectors (SNSPDs)' (57 chars)

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shortdescription => protected'Superconducting Nanowire Single-Photon Detectors (SNSPDs) are cutting-edg
e devices that enable the reliable detection of individual photons. They are
formed by nano-patterning thin superconducting films to form nanowires wire
s.  When operated at cryogenic temperatures, they deliver unmatched per
formance for quantum light detection with high efficiency, low noise, phonon
-number resolution and picosecond photon timing precision. Thanks to their s
peed and sensitivity across a wide range of wavelengths spanning the visible
to infrared, SNSPDs are a key technology for quantum communication, secure
data transfer, advanced imaging, and fundamental scientific research.  
In the WSI we work closely with <a href="https://munich-quantum-instruments.
com" title="Munich Quantum Instruments">Munich Quantum Instruments GmbH</a>
and the QEC Group led by <a href="https://www.ee.cit.tum.de/qec/home/" title
="Kai Müller">Kai Müller</a> in the framework of several third-party researc
h projects developing the materials technologies for SNSPDs made from polycr
ystalline superconducting thin films such as MoSi and NbTiN, as well as emer
gent van der Waals superconductors like NbSe2.  We aim to un
derstand the microscopic mechanisms governing the photo-detection process an
d apply e.g. local He-ion irradiation to enhance detector performance. &nbsp
;Detectors are integrated into quantum photonic circuits with much scope for
emergent quantum photonic technologies.   ' (1501 chars)

description => protected'Longer Text Description' (30 chars)

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title => protected'Quantum Sensing' (15 chars)

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title => protected'Munich Initiative for Cross-Correlative Spin Microscopy (MICroCoSM)' (67 chars)

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shortdescription => protected'The overarching goal of the Munich Initiative for Cross-Correlati
ve Spin Microscopy (MICroCoSM) is to facilitate the study of nanosc
ale quantum materials and hybrid quantum systems using the high-resolution -
and crucially - the multi-modal spectroscopy offered by tip-based nitrogen
vacancy (NV) quantum sensing.  The unique system installed in the labs
of WSI moves the boundary of the experimental state-of-the-art by enabling tip-based, time resolved single spin spectroscopy at low temperatures in h
igh magnetic fields.  This is done using a low-temperature version
of the <a href="https://qnami.ch/portfolio/proteusq/" title="ProteusQ LM">Pr
oteusQ </a>scanning NV microscope from <a href="https://qnami.ch" title="Qna
mi">Qnami</a> as a Spin-based Quantum Light Microscope (SQLM).  It prov
ides nanoscale access to magnetic properties of nano-materials subject to el
ectrical / optical perturbations.  Feel free to reach out to <a href="m
ailto:jj.finley@tum.de?subject=Interest%20in%20SQLM" title="SQLM">Prof. Finl
ey</a> if you are interested!' (1097 chars)

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title => protected'Nanoscale quantum magnetometry' (30 chars)

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shortdescription => protected'The Nanoscale Quantum Magnetometer is a scanning pro
be microscope based on a single nitrogen vacancy (NV) center implanted in a
diamond tip. The spin and optical dipole of the NV center can be used to mea
sure stray electric and magnetic fields with nanoscale spatial resolution an
d exceptional dynamic range. The overarching goal of this instrument is to e
nable the study of nanoscale quantum materials and hybrid quantum systems us
ing the high-resolution - and crucially - the multi-modal spectroscopy offer
ed by tip-based NV quantum sensing. The unique proposed system moves the bou
ndary of the experimental state-of-the-art by enabling tip-based, time re
solved single spin spectroscopy at low temperatures in high magnetic fields. These capabilities are unique but necessary in order to manipulate and
investigate the spin-and charge configurations of quantum matter. Moreover,
the instrument has a sophisticated optical design to enable advanced opti
cal spectroscopy experiments to correlate in real-time the nanoscale NV
probe measurements with global observables. This project will enable complet
ely new insight into the challenging but critical phase space from single pa
rticle interactions to a global quantum phase, and therefore overcomes the m
ain experimental roadblocks to understand emergence in quantum matter. 
' (1372 chars)

description => protected'A conventional approach to study many-body systems a
t the single-particle level would be with a series of specialized scanning t
ip microscopes, capable of probing many of the most fundamental properties o
f condensed matter systems, from sample morphology to magnetism, optical con
ductivity, electronic energy levels, etc. However, this approach requires di
fferent instruments or at least different probe tips, which practically ofte
n times bring along incompatible system or sample requirements. Cruc
ially, however, the conventional approach is blind to the fact that emergent
phases are intrinsically linked to all of the above – simultaneously -</str
ong> and most conventional methods can only probe static properties. Only an
NV-based system is able to combine all sample properties to fully understan
d emergence in solids.' (862 chars)

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title => protected'Group-IV Quantum Emitters' (25 chars)

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title => protected'Hexagonal Silicon Germanium' (27 chars)

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shortdescription => protected'By far the most important chip materials are silicon (Si) and germanium (
Ge), accounting for ~90% of global demand, and entirely dominating the elect
ronics industry. Silicon chips could be much faster and more energy efficien
t if they operated with light. Silicon, germanium, and their alloys do not e
fficiently emit light in their naturally occurring, cubic, crystal form due
to their indirect bandgap.  However, a newly discovered allotrope of Si
Ge - hexagonal SiGe - efficiently emits light, holding much
promise for silicon based classical and quantum photonic technologies.&nbsp
;' (613 chars)

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descriptivename => protected'Nanotechnology and Nanomaterials' (32 chars)

description => protected'Structuring materials with atomic precision is the ultimate goal of nanot
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r quantum electronics, spintronics, optoelectronics, and photonics, as well
as for energy conversion applications. Our chair explores the possibility to
structure materials on an atomic level and to explore the fundamental physi
cal properties of atomistic 2D materials with a specific focus on semiconduc
ting nanomaterials for future information and energy conversion technologies
. We follow four main research directions: <ul><li><a href="t3:
//record?identifier=topic&uid=20">Single-atom circuits</a><
/li><li><a href="t3://record?identifier=topic&uid=23">Topological
electronics and materials</a></li><li><a href="t3://record?identifier
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ndensates</a></li><li><a href="t3://record?identifier=topic&uid=2
2">Femtosecond on-chip electronics</a></li></ul>' (1049 chars)

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description7 => protected'We are always looking for interested Bachelor, Master and PhD students. P
lease, contact Prof. Holleitner and/or Dr. Kastl for position openings.' (151 chars)

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shortdescription => protected'Increasing the interaction strength between quasi-particles in solid-stat
e materials can cause strong correlations, collective phenomena and the tran
sition to macroscopic quantum phases, such as a Bose-Einstein condensate. He
terostructures made of semiconducting 2D materials, such as MoSe2
and WSe2, are ideal systems to realize interacting exciton ensem
bles, because they provide large exciton binding energies, long photolumines
cence lifetimes, as well as a permanent exciton dipole. The latter allows th
e manipulation of the exciton ensembles, e.g. via electric fields. Recently,
we have reported on several signatures regarding photoluminescence intensit
y, linewidth, as well as spatial and temporal coherences in accordance with
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ing studies want to explore further predicted phases, such as an excitonic s
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Berlin).' (1076 chars)

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shortdescription => protected'We generate optically active defects in atomically thin 2D materials on a
spatial scale of below 10 nm, such that scalable opto/electronics based on
individual atomic states seems at reach. We use a helium-ion microscope (HIM
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materials with more than a thousand different materials and is compatible w
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vidual atomic defects. At the same time, fundamental processes, such as the
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calized states in a Fermion boson mixture are experimentally accessible.
Collaborators: Jonathan Finley (TUM), Kai Müller (TUM), Nicolas Leither
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shortdescription => protected'We are heading the Center for Nanotechnologies and Nanomaterials (ZNN), w
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f TUM. Students, researchers, and scholars from the greater scientific Munic
h area have access to state-of-the-art nanolithography and nanoanalytic inst
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m-ion-beam lithography.' (483 chars)

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title => protected'Towards femtosecond on-chip electronics' (39 chars)

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shortdescription => protected'The vision of this research topic is to generate electric current pulses
with a duration of only a few femtoseconds for an on-chip signal conversion
at the interface between electronics and optics, the so-called THz-gap. For
signal generation we use amongst others, photo-emission processes, such as m
ultiphoton absorption and strong field tunnel processes in plasmonic nanocon
tacts; but also femtosecond processes within solid state materials. The sign
al propagation occurs via electromagnetic THz modes in coplanar strip conduc
tors. For the on-chip THz-detection, we are working on an electrical detecti
on on the 100 fs scale and faster. Currently we reach 350 fs by using the re
laxation dynamics in amorphous silicon photo-switches. Our group manufacture
s all circuits in our own laboratory, and we use phase-stable femtosecond la
sers to drive the on-chip THz circuits coherently. Intriguingly, atomically
thin 2D materials can be integrated into the THz circuits without much effor
t, such that the 2D materials can act as functional THz modulators. In the s
ame way, the electron and heat dynamics in the 2D materials can be investiga
ted on a femto- to picosecond timescale. Collaborator: Reinhard Kien
berger (TUM).' (1233 chars)

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title => protected'Topological electronics and materials' (37 chars)

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shortdescription => protected'Topological materials are very promising for future opto/electronic circu
its, since computing schemes can be envisaged where e.g. information-carryin
g surface states are protected by topology. Van der Waals materials and thei
r heterostructure are an ideal platform to engineer and explore topological
states. On the one hand, one can control and break the relevant symmetries o
f the Hamiltonian at will by interfacing different van der Waals materials w
ith different symmetries. On the other hand, we can directly address the sym
metry of the electron-Bloch states in the van der Waals crystal e.g. by exte
rnal electric fields. In our research, we explore a wide range of non-trivia
l, i.e. topological quantum phenomena. The research is headed by Dr. Christo
ph Kastl. Collaborator: Marko Burghard (MPI Stuttgart).' (827 chars)

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description => protected'Understanding and controlling the interaction of light, charge, and mater
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able energy technologies. To address these challenges, we design and develop
advanced semiconducting materials and functional interfaces, with a focus o
n thin films and their heterostructures for solar energy conversion, electro
catalysis, and optoelectronics. Through our research, we aim to un
cover and direct optical excitations, charge carrier transport mechanis
ms, and interfacial dynamics. To gain new insights into these fund
amental processes, we combine advanced deposition methods, includi
ng reactive sputtering, atomic layer deposition, and molecular beam epitaxy,
with a comprehensive suite of (in situ) structural, ele
mental, and optoelectronic characterization tools. This integrated approach
enables us to interrogate and guide complex light-to-charge and charge-
to-chemical transformation pathways that underlie the functional characteris
tics of emerging optoelectronic and energy conversion systems.' (1130 chars)

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title => protected'Discovery and development of advanced thin film semiconductors' (62 chars)

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shortdescription => protected'Thin film semiconductors based on nitrides, oxynitrides, and oxides serve
as versatile platforms for tailoring electronic and optical properties of m
aterials. By leveraging advanced deposition techniques, such as reactive spu
tter deposition, molecular beam epitaxy, and solution-based processing, we e
xplore novel material compositions with precisely controlled structures. A k
ey focus of our research is the comprehensive characterization of these mate
rials, including their elemental composition and atomic bonding environments
, electronic structures, and excited state characteristics using a combinati
on of lab- and synchrotron-based techniques. With this suite of complementar
y experimental tools, we investigate defects, doping strategies, and charge
transport dynamics to understand and tune optical and electronic properties.
These insights are crucial for controlling the functional properties of the
se materials for applications that include photoelectrochemical energy conve
rsion, solar cells, and sustainable electronic devices. ' (1053 chars)

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title => protected'In situ & operando spectroscopy at reactive interfaces' (54 chars)

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shortdescription => protected'To unlock the full potential of functional materials, it is essential to
study their properties under realistic operating conditions. Our research fo
cuses on the development of in situ and operando spectroscopic techniques th
at provide real-time insights into the structural, electronic, and chemical
dynamics of thin films, electrocatalysts, and semiconductor systems. In part
icular, we employ near-ambient pressure X-ray photoelectron spectroscopy (NA
P-XPS) to probe surface chemistry in reactive environments, transient absorp
tion spectroscopy (TAS) to track charge carrier and electrochemical dynamics
, Fourier-transform infrared (FTIR) spectroscopy to monitor molecular vibrat
ions and reaction intermediates, and Raman spectroscopy to analyze structura
l transformations of materials driven away from equilibrium. These technique
s allow us to correlate key energy conversion performance metrics with the e
lectronic structure, defect states, and reaction mechanisms in dynamic envir
onments. Our approach bridges fundamental materials science with innovative
energy conversion concepts, enabling the design of more efficient and stable
energy materials.' (1162 chars)

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title => protected'Tailored (photo)electrochemical interfaces' (42 chars)

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shortdescription => protected'The performance of advanced energy materials is critically determined by
their interfaces. In (photo)electrochemical systems, efficient charge transf
er relies on the precise design of both solid-solid and solid-liquid interfa
ces. Our research focuses on tailoring these interfaces at the atomic- and n
anoscale to precisely guide efficient energy conversion processes. A key asp
ect of this research is based on the alignment of energy levels at heterojun
ctions, which governs selective charge injection and extraction. In addition
, we investigate semiconductor-liquid junctions, where interfacial electric
fields and surface states play a crucial role in dictating reaction kinetics
. Beyond material properties, we study how microenvironments around electroc
atalysts – including local pH, ion distribution, and solvation effects – can
influence reaction selectivity. These insights are applied to the developme
nt of materials for sustainable generation of chemicals from sunlight, with
tailored interfacial properties enabling accelerated charge transfer, enhanc
ed reaction selectivity, and improved conversion efficiency.' (1128 chars)

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title => protected'Ultrathin functional materials via atomic layer deposition' (58 chars)

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shortdescription => protected'From tunable dielectrics integrated into nanoscale electronic devices to
multifunctional coatings that promote efficient solar-to-chemical energy con
version, we make extensive use of atomic layer deposition (ALD) to precisely
engineer interfaces, design novel heterostructures, and introduce defined f
unctionalities at surfaces. Within this research, we develop novel ALD proce
sses and materials, guided by in situ spectroscopic ellipsometry and mass sp
ectrometry that offer real-time insights into nucleation dynamics, growth ki
netics, defect formation, and film properties. Moving beyond traditional app
roaches, we explore advanced ALD strategies by, for example, integrating pla
sma-surface interactions to tune interfacial chemical and electronic propert
ies, introducing external stimuli to achieve area-selective growth, and tail
oring reaction conditions to shape nanoscale morphologies. By advancing ALD-
based methods for precise interface and material control, our work contribut
es to the development of next-generation electronic, energy, and catalytic s
ystems in which nanoscale structure-property relationships are critical.' (1140 chars)

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WSI dev: Research overview